The crystal structure, optical properties, electronic band structure, laser damage threshold, and hardness of the GSP crystal were comprehensively investigated. In this work, a Gd-based orthophosphate crystal, GdSr 3(PO 4) 3, (GSP), and a Nd 3+-doped GdSr 3(PO 4) 3 crystal, (Nd:GSP), were obtained by the Czochralski method. Disordered crystals have attracted immense attention for the generation of ultrashort laser pulses due to their good thermomechanical characteristics and wide emission bandwidths.
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